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THz Magneto-electric atomic rotations in the chiral compound Ba$_3$NbFe$_3$Si$_2$O$_{14}$

Published 7 Mar 2013 in cond-mat.str-el and cond-mat.mtrl-sci | (1303.1706v2)

Abstract: We have determined the terahertz spectrum of the chiral langasite Ba$3$NbFe$_3$Si$_2$O${14}$ by means of synchrotron-radiation measurements. Two excitations are revealed that are shown to have a different nature. The first one, purely magnetic, is observed at low temperature in the magnetically ordered phase and is assigned to a magnon. The second one persits far into the paramagnetic phase and exhibits both an electric and a magnetic activity at slightly different energies. This magnetoelectric excitation is interpreted in terms of atomic rotations and requires a helical electric polarization.

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