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The mode-locking transition of random lasers

Published 12 Apr 2013 in physics.optics | (1304.3652v1)

Abstract: The discovery of the spontaneous mode-locking of lasers, i.e., the synchronous oscillation of electromagnetic modes in a cavity, has been a milestone of photonics allowing the realization of oscillators delivering ultra-short pulses. This process is so far known to occur only in standard ordered lasers with meter size length and only in the presence of a specific device (the saturable absorber). Here we demonstrate that mode-locking can spontaneously arise also in random lasers composed by micronsized laser resonances dwelling in intrinsically disordered, self-assembled clusters of nanometer-sized particles. Moreover by engineering a novel mode-selective pumping mechanism we show that it is possible to continuously drive the system from a configuration in which the various excited electromagnetic modes oscillate in the form of several, weakly interacting, resonances to a collective strongly interacting regime. By realizing the smallest mode-locking device ever fabricated, we open the way to novel generation of miniaturized and all-optically controlled light sources.

Citations (195)

Summary

Analysis of Mode-Locking Transition in Random Lasers

The study presented in "The mode-locking transition of random lasers" explores the spontaneous occurrence of mode-locking in random lasers (RLs), a feature traditionally associated with ordered laser systems utilizing saturable absorbers. This paper delves into the complexities of RLs, which are composed of disordered materials that can amplify light when optically pumped. By demonstrating mode-locking in RLs, the authors introduce potential advancements in the miniaturization and optical control of laser devices.

In conventional laser systems, mode-locking synchronizes electromagnetic modes within the laser cavity, producing ultra-short pulses. Typically, this process is achieved through the use of saturable absorbers in meter-sized cavities. The primary contribution of this paper lies in extending the concept of mode-locking to RLs, which are characterized by their disordered structure and micron-sized resonances.

The authors employ a novel mode-selective pumping scheme to explore the transition from an incoherent feedback random laser (IFRL) to a resonant feedback random laser (RFRL). By varying the spatial shape of the pumping beam, they effectively direct the amplification to selective modes within the RL. This allows for controlled transitions between different lasing regimes.

Key experimental results of the paper include:

  • The transition from RFRL, exhibiting sharp spectral peaks associated with distinct modes, to IFRL, characterized by a smooth emission spectrum reminiscent of classic laser systems.
  • The introduction of a "spikiness" parameter (S) to quantify the transition. S was found to vary with the angular aperture ($\Theta$) of the pumped area, indicating the extent of mode interaction.
  • A strong correlation between mode intensities was observed as the system transitioned to IFRL, signifying the onset of a mode-locked state.

Theoretical implications are discussed using coupled mode theory (CMT), which corroborates the experimental findings by modeling the interaction between different laser modes subjected to varying degrees of coupling. The numerical simulations reveal how increasing the number of coupled modes leads to phase synchronization—a hallmark of mode-locking.

Practically, this work paves the way for the development of compact and tunable laser sources without the need for additional mode-locking components. The transition between distinct random lasing regimes through external control presents opportunities for novel optical devices in photonics, potentially impacting telecommunications, sensing, and medical applications.

Theoretically, the findings bridge concepts from the physics of complex systems and laser science, suggesting that RLs may serve as experimental platforms for studying phenomena akin to Bose-Einstein condensation and the statistical physics of disordered systems.

Future research directions may explore the influence of different material compositions on the mode-locking process in RLs, the potential for electrically-pumped RLs, and broader integration into photonic circuits.

In essence, this paper significantly enhances the understanding of RLs by uncovering the conditions under which their modes can spontaneously lock, offering new insights into both photonic applications and fundamental light-matter interactions.

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