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Broadband Photovoltaic Detectors based on an Atomically Thin Heterostructure

Published 8 Jan 2016 in cond-mat.mtrl-sci and cond-mat.mes-hall | (1601.01814v1)

Abstract: Van der Waals junctions of two-dimensional materials with an atomically sharp interface open up unprecedented opportunities to design and study functional heterostructures. Semiconducting transition metal dichalcogenides have shown tremendous potential for future applications due to their unique electronic properties and strong light-matter interaction. However, many important optoelectronic applications, such as broadband photodetection, are severely hindered by their limited spectral range and reduced light absorption. Here, we present a p-g-n heterostructure formed by sandwiching graphene with a gapless bandstructure and wide absorption spectrum in an atomically thin p-n junction to overcome these major limitations. We have successfully demonstrated a MoS2-graphene-WSe2 heterostructure for broadband photodetection in the visible to short-wavelength infrared range at room temperature that exhibits competitive device performance, including a specific detectivity of up to 1011 Jones in the near-infrared region. Our results pave the way toward the implementation of atomically thin heterostructures for broadband and sensitive optoelectronic applications.

Citations (319)

Summary

  • The paper demonstrates a novel p-g-n heterostructure design that integrates graphene with MoS₂ and WSe₂ to achieve broadband photodetection from visible to infrared wavelengths.
  • It reports key metrics including a specific detectivity of up to 10¹¹ Jones in the near-infrared and a photoresponsivity of approximately 10 A/W in the visible spectrum.
  • The results suggest promising applications in imaging, sensing, and telecommunications, offering a viable, room-temperature alternative to conventional cryogenic detectors.

Overview of Broadband Photovoltaic Detectors Based on an Atomically Thin Heterostructure

The paper presents a significant advancement in the development of broadband photovoltaic detectors using atomically thin heterostructures. The work focuses on leveraging van der Waals junctions comprised of two-dimensional (2D) materials to innovate optoelectronic applications, addressing the challenges associated with limited spectral range and reduced light absorption in existing technologies.

Key Contributions

The authors introduce a novel p-g-n heterostructure, which utilizes graphene—a material with a gapless band structure—sandwiched between MoS₂ and WSe₂ layers to form an atomically thin p-n junction. The device demonstrates broadband photodetection capabilities from the visible to the short-wavelength infrared range at room temperature. The strategic use of graphene capitalizes on its wide absorption spectrum, while the p-n junction provides an efficient built-in electric field to separate photoexcited charge carriers.

Numerical Findings

A notable performance metric of the reported MoS₂-graphene-WSe₂ heterostructure is its specific detectivity, reaching up to 10¹¹ Jones in the near-infrared region. The device exhibits a high photoresponsivity of approximately 10 A/W in the visible spectrum. These results are indicative of its potential for integration into commercial optoelectronic applications without requiring complex cooling systems.

Implications and Prospects

The successful fabrication and characterization of this heterostructure underscore the capabilities of 2D materials in enhancing the functionality of photodetectors. This work paves the way for the broad application of atomically thin van der Waals heterostructures in fields such as sensing, imaging, and telecommunications. The device's performance suggests it could serve as a viable alternative to existing photodetectives, particularly those like InGaAs detectors, which typically operate at cryogenic temperatures.

Looking ahead, further enhancements in device performance are plausible through optimization of material properties and junction engineering. Adjustments in doping levels and Fermi-level tuning could lead to improved responsivity and detectivity. Moreover, the underlying principles of this research can be extrapolated to design versatile optoelectronic systems with heightened integration capabilities.

Conclusion

This research articulates a promising step forward in the field of broadband photodetectors through the innovative use of atomically thin heterostructures. The incorporation of 2D materials like graphene within p-n junctions has demonstrated substantial improvements in light sensitivity and spectral range, establishing a foundation for future enhancements and applications in advanced optoelectronic devices.

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