Spin and charge caloritronics in bilayer graphene flakes with magnetic contacts

Abstract: We investigate the coupling of spin and thermal currents as a means to rise the thermoelectric efficiency of nanoscale graphene devices. We consider nanostructures composed of overlapping graphene nanoribbons with ferromagnetic contacts in different magnetic configurations. Our results show that the charge Seebeck effect is greatly enhanced when the magnetic leads are in an antiparallel configuration, due to the enlargement of the transport gap. However, for the optimization of the charge figure of merit ZT it is better to choose a parallel alignment of the magnetization in the leads, because the electron-hole symmetry is broken in this magnetic configuration. We also obtain the spin-dependent Seebeck coefficient and spin figure of merit. In fact, the spin ZT can double its value with respect to the charge ZT for a wide temperature range, above 300 K. These findings suggest the potential value of graphene nanosystems as energy harvesting devices employing spin currents.