Photoinduced topological phase transitions in strained black phosphorus

Abstract: Photoinduced topological phase transitions (TPTs) in black phosphorous (BP) under compressive strain were investigated by combining Floquet theory and first-principles calculations. Intriguing photo-dressed electronic states including Floquet-Dirac semimetals and Floquet topological insulators have been identified, which can be feasibly engineered by changing the direction, intensity and frequency of incident laser. Remarkably, tunable TPT from type-I to type-II Floquet-Dirac fermions can be realized by irradiating circularly polarized laser (CPL), with an origin rooted in optical Stark effect. Furthermore, the photoinduced Floquet-Dirac phases is shown to host topological surface states that exhibit nonequilibrium electron transport in a direction locked by the helicity of CPL. This work provides useful guidance for experimental observation of Floquet TPTs, and extends optoelectrionic applications of BP to nonequilibrium regime.