Coherent photon coincidence spectroscopy of single quantum systems

Abstract: Non-equilibrium photon correlations of coherently excited single quantum systems can reveal their internal quantum dynamics and provide spectroscopic access. Here we propose and discuss the fundamentals of a coherent photon coincidence spectroscopy based on the application of laser pulses with variable delay and the detection of an time-averaged two-photon coincidence rate. For demonstration, two simple but important cases, i.e., an exciton - biexciton in a quantum dot and two coupled quantum emitters, are investigated based on quantum dynamics simulations demonstrating that this nonlinear spectroscopy reveals information specific to the particular single quantum system.