Bonding and antibonding modes in metal-dielectric-metal plasmonic antennas for dual-band applications

Abstract: Resonant optical antennas supporting plasmon polaritons (SPPs) - collective excitations of electrons coupled to electromagnetic fields in a medium - are relevant to sensing, photovoltaics, and light-emitting devices, among others. Due to the SPP dispersion, a conventional antenna of fixed geometry, exhibiting a narrow SPP resonance, cannot simultaneously operate in two different spectral bands. In contrast, here it is demonstrated that in metallic disks, separated by a nanometric spacer, the hybridized antibonding SPP mode stays in the visible range, while the bonding one can be pushed down to the mid-infrared range. Such an SPP dimer can sense two materials of nanoscale volumes, whose fingerprint central frequencies differ by a factor of 5. Additionally, the mid-infrared SPP resonance can be tuned by employing a phase-change material (VO2) as a spacer. The dielectric constant of the phase-change material is controlled by heating the material at the frequency of the antibonding optical mode. These findings open the door to a new class of optoelectronic devices able to operate in significantly different frequency ranges in the linear regime, and with the same polarization of the illuminating wave.