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Delayed $^{160}$Tb radioactivity buildup due to $^{159}$Tb(n,$^2$n) nuclear reaction products transformation and subsequent fusion

Published 25 Jun 2021 in nucl-ex | (2106.14661v5)

Abstract: This paper deals with the formation of a bound dineutron in the outgoing channel of the ${159}$Tb(n,$2$n)${158g}$Tb nuclear reaction followed by assumed transformations of this reaction products ${159g}$Tb and $2$n. Such nuclear processes were studied in detail from the point of view of ${160}$Tb / ${160}$Dy / ${160}$Ho amount of nuclei versus time dependence. Some signs of fusion process between heavier nuclei (${158}$Tb and/or ${158}$Gd) and the deuteron, that is a bound dineutron decay product, were detected as unexpected increasing of 879.38 keV gamma-ray peak count rate due to ${160}$Dy gamma-transitions. The mathematical model, including three systems of differential equations, was developed to describe the experimental data. This development requires a reasonable estimate of the half-life of a bound dineutron, which was found to be equal 5,877 s as an upper limit. We mathematically modeled the experimentally observed delayed in time buildup of the ${160}$Tb radioactivity with a maximum at about 495 d since the neutron irradiation completion of the Tb sample, based on the similarity with the parent-daughter nuclei radioactivity decay and nuclear accumulation processes.

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