Photoluminescence of double quantum wells: asymmetry and excitation laser wavelength effects

Abstract: Circularly polarized photoluminescence (PL) spectroscopy measured at 19 K on GaAs/AlGaAs symmetric and asymmetric double quantum wells (DQW) is reported. The PL is obtained by exciting the sample with a circularly polarized (left or right) laser in order to create an initial unbalanced distribution of electron spins in the conduction band and, in this way, obtain the electron spin lifetime $\tau_s$. The effects of the excitation laser wavelength were estimated by exciting with laser wavelengths of 701.0 nm, 787.0 nm, 801.5 nm and 806.5 nm. The increase of $\tau_s$ with the excitation wavelength is attributed to the lower initial quasi-momentum $\bf{k}$ of the excited carriers, which also reduces spin-orbit relaxation processes. $\tau_s$ was found to be higher in asymmetric DQWs: this is attributed to the wider QWs in these samples, which reduces spin relaxation due to the Dresselhaus mechanism. In addition, we also detected a smaller contribution from the Rashba mechanism by comparing samples with built-in electric fields of different orientations defined by doped barrier layers.