Flow induced rigidity percolation in shear thickening suspensions

Abstract: Discontinuous shear thickening (DST) is associated with a sharp rise of a suspension's viscosity with increasing applied shear rate. A key signature of DST, highlighted in recent studies, is the very large fluctuations of the measured stress as the suspension thickens. A clear link between microstructural development and the dramatic increase of the stress fluctuations has not been established yet. To identify the microstructural underpinnings of this behavior, we perform simulations of sheared dense suspensions. By analyzing particle contact networks, we identify a subset of constrained particles that contribute directly to the rapid rise in viscosity and the large stress fluctuations. Indeed, both phenomena can be explained by the growth and percolation of constrained particle networks -- in direct analogy to rigidity percolation. A finite size scaling analysis confirms this is a percolation phenomenon and allows us to estimate the critical exponents. Our findings reveal the specific microstructural transition that underlies DST.