Trapping and Ground-State Cooling of a Single H$_2^+$

Abstract: We demonstrate co-trapping and sideband cooling of a H$2^+$ - $^9$Be$^+$ ion pair in a cryogenic Paul trap. We study the chemical lifetime of H$_2^+$ and its dependence on the apparatus temperature, achieving lifetimes of up to $11^{+6}{-3}$ h at 10 K. We demonstrate cooling of two of the modes of translational motion to an average phonon number of 0.07(1) and 0.05(1), corresponding to a temperature of 22(1) $\mu$K and 55(3) $\mu$K respectively. Our results provide a basis for quantum logic spectroscopy experiments of H$_2^+$, as well as other light ions such as HD$^+$, H$_3^+$, and He$^+$.