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Oscillations in the magnetothermal conductivity of $\boldsymbolα$-RuCl$_3$: Evidence of transition anomalies

Published 12 Jan 2023 in cond-mat.str-el | (2301.05254v1)

Abstract: The 2D layered insulator $\alpha$-RuCl$3$ is a candidate material for a quantum spin-liquid state, which may be realized when a magnetic field suppresses the antiferromagnetic order present at low temperature. Oscillations in the field dependence of the thermal conductivity, observed for an in-plane magnetic field $B$ up to a critical field $B{\star}$, have been attributed to exotic charge-neutral fermions, viewed as evidence of a quantum spin-liquid state between the critical field $B{c}$ $\simeq 7$ T at which the antiferromagnetic phase ends and $B{\star}$. Here we report measurements of the thermal conductivity of $\alpha$-RuCl$3$ as a function of magnetic field up to 15 T applied in two distinct in-plane directions: parallel and perpendicular to the Ru-Ru bond. We find that the number of oscillations between $B{c}$ and $B{\star}$ is the same for the two field directions even though the field interval between $B_{c}$ and $B{\star}$ is different. In other words, the period of the oscillations is controlled by the transition fields $B_{c}$ and $B{\star}$. We conclude that these are not true oscillations -- coming from putative fermions in a spin-liquid state -- but anomalies associated with a sequence of magnetic transitions.

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