Orbital Gravito-Magnetoelectric response and Orbital magnetic quadrupole moment correction

Abstract: The magnetoelectric effect has been actively studied in multiferroics since the first observation in an antiferromagnetic, $\mathrm{Cr_2O_3}$. This effect appears in systems without spatial inversion symmetry and time-reversal symmetry and is sensitive to detecting magnetic quadrupole moments. It is often discussed as inducing spin magnetizations; however, the orbital magnetoelectric effect in metals has recently attracted much attention since its observation in $\mathrm{MoS_2}$ and twisted bilayer graphene. In this work, we propose the full quantum formalism for the temperature gradient induced-orbital magnetoelectric effect (orbital gravito-ME effect). The effect consists of two parts, i.e., an extrinsic part and an intrinsic part. We demonstrate that the intrinsic part needs a correction from the orbital magnetic quadrupole moment besides the usual Kubo formula to avoid an unphysical divergence at zero temperature and to satisfy the Mott relation. Furthermore, we show the classification table with the magnetic point group for the intrinsic and extrinsic effects. Finally, we analyze the intrinsic part in a $\mathcal{PT}$-symmetric model exhibiting an orbital magnetization order, i.e., a loop current order, and demonstrate the enhancement near Dirac points. We believe that these results will contribute to the detection and usage of orbital magnetic moments beyond spin moments.