A Reversed Inverse Faraday Effect

Abstract: The inverse Faraday effect is a magneto-optical process allowing the magnetization of matter by an optical excitation carrying a non-zero spin of light. In particular, a right circular polarization generates a magnetization in the direction of light propagation and a left circular polarization in the opposite direction to this propagation. We demonstrate here that by manipulating the spin density of light, i.e., its polarization, in a plasmonic nanostructure, we generate a reversed inverse Faraday effect. A right circular polarization will generate a magnetization in the opposite direction of the light propagation, a left circular polarization in the direction of propagation. Also, we demonstrate that this new physical phenomenon is chiral, generating a strong magnetic field only for one helicity of the light, the opposite helicity producing this effect only for the mirror structure. This new optical concept opens the way to the generation of magnetic fields with unpolarized light, finding application in the ultrafast manipulation of magnetic domains and processes, such as spin precession, spin currents, and waves, magnetic skyrmion or magnetic circular dichroism, with direct applications in data storage and processing technologies.