Tailoring topological band properties of twisted double bilayer graphene: effects due to spin-orbit coupling
Abstract: Our theoretical study unfolds the topological phase transitions (within bands of the Moir\'e super-lattice) in small angle twisted double bilayer graphene (tDBLG) under the influence of external gate voltage and intrinsic spin-orbit coupling (SOC) for both AB-AB and AB-BA stacking configurations. Utilizing a low-energy continuum model, we investigate the band structure and perform a comprehensive topological characterization of the system by analysing the direct band gap closing as well as various Chern numbers. In the absence of SOC, the tDBLG exhibits characteristics of a valley Hall insulator. However, in the presence of SOC, we observe a transition to a quantum spin Hall insulator state and band topology emerges in the parameter spaces of non-topological regime without SOC. Furthermore, we conduct a comparative analysis between untwisted double bilayer graphene and tDBLG to assess the impact of twisting on the system's properties. Our findings reveal the construction of topological phase diagrams that showcase distinct phases arising from changes in the twist angle compared to the untwisted case. These phase diagrams provide valuable insights into the diverse topological phases achievable in tDBLG with SOC. Our findings contribute to the understanding of the interplay between small twist angle, SOC, and external electric field on the topological band properties of twisted multilayer graphene systems.
- A. K. Geim and K. S. Novoselov, “The rise of graphene,” Nature Materials 6, 183–191 (2007).
- A. H. Castro Neto, F. Guinea, N. M. R. Peres, K. S. Novoselov, and A. K. Geim, “The electronic properties of graphene,” Rev. Mod. Phys. 81, 109–162 (2009).
- E. McCann and M. Koshino, “The electronic properties of bilayer graphene,” Reports on Progress in Physics 76, 056503 (2013).
- H. Min and A. H. MacDonald, “Electronic Structure of Multilayer Graphene,” Progress of Theoretical Physics Supplement 176, 227–252 (2008).
- J. M. B. Lopes dos Santos, N. M. R. Peres, and A. H. Castro Neto, “Graphene bilayer with a twist: Electronic structure,” Phys. Rev. Lett. 99, 256802 (2007).
- S. Shallcross, S. Sharma, and O. A. Pankratov, “Quantum interference at the twist boundary in graphene,” Phys. Rev. Lett. 101, 056803 (2008).
- G. Li, A. Luican, J. M. B. Lopes dos Santos, A. H. Castro Neto, A. Reina, J. Kong, and E. Y. Andrei, “Observation of van hove singularities in twisted graphene layers,” Nature Physics 6, 109–113 (2010).
- R. Bistritzer and A. H. MacDonald, “Moiré bands in twisted double-layer graphene,” Proceedings of the National Academy of Sciences 108, 12233–12237 (2011).
- P. Moon, Y.-W. Son, and M. Koshino, “Optical absorption of twisted bilayer graphene with interlayer potential asymmetry,” Phys. Rev. B 90, 155427 (2014a).
- M. Koshino, N. F. Q. Yuan, T. Koretsune, M. Ochi, K. Kuroki, and L. Fu, “Maximally localized wannier orbitals and the extended hubbard model for twisted bilayer graphene,” Phys. Rev. X 8, 031087 (2018).
- Y. Cao, V. Fatemi, A. Demir, S. Fang, S. L. Tomarken, J. Y. Luo, J. D. Sanchez-Yamagishi, K. Watanabe, T. Taniguchi, E. Kaxiras, R. C. Ashoori, and P. Jarillo-Herrero, “Correlated insulator behaviour at half-filling in magic-angle graphene superlattices,” Nature 556, 80–84 (2018a).
- Y. Cao, V. Fatemi, S. Fang, K. Watanabe, T. Taniguchi, E. Kaxiras, and P. Jarillo-Herrero, “Unconventional superconductivity in magic-angle graphene superlattices,” Nature 556, 43–50 (2018b).
- H. C. Po, L. Zou, A. Vishwanath, and T. Senthil, “Origin of mott insulating behavior and superconductivity in twisted bilayer graphene,” Phys. Rev. X 8, 031089 (2018).
- Z. Song, Z. Wang, W. Shi, G. Li, C. Fang, and B. A. Bernevig, “All magic angles in twisted bilayer graphene are topological,” Phys. Rev. Lett. 123, 036401 (2019).
- M. Xie and A. H. MacDonald, “Nature of the correlated insulator states in twisted bilayer graphene,” Phys. Rev. Lett. 124, 097601 (2020).
- T. M. R. Wolf, J. L. Lado, G. Blatter, and O. Zilberberg, “Electrically tunable flat bands and magnetism in twisted bilayer graphene,” Phys. Rev. Lett. 123, 096802 (2019).
- Z.-D. Song and B. A. Bernevig, “Magic-angle twisted bilayer graphene as a topological heavy fermion problem,” Phys. Rev. Lett. 129, 047601 (2022).
- S. Wu, Z. Zhang, K. Watanabe, T. Taniguchi, and E. Y. Andrei, “Chern insulators, van hove singularities and topological flat bands in magic-angle twisted bilayer graphene,” Nature Materials 20, 488–494 (2021).
- K. P. Nuckolls, M. Oh, D. Wong, B. Lian, K. Watanabe, T. Taniguchi, B. A. Bernevig, and A. Yazdani, “Strongly correlated chern insulators in magic-angle twisted bilayer graphene,” Nature 588, 610–615 (2020).
- M. Oh, K. P. Nuckolls, D. Wong, R. L. Lee, X. Liu, K. Watanabe, T. Taniguchi, and A. Yazdani, “Evidence for unconventional superconductivity in twisted bilayer graphene,” Nature 600, 240–245 (2021).
- J.-X. Lin, Y.-H. Zhang, E. Morissette, Z. Wang, S. Liu, D. Rhodes, K. Watanabe, T. Taniguchi, J. Hone, and J. I. A. Li, “Spin-orbit–driven ferromagnetism at half moiré filling in magic-angle twisted bilayer graphene,” Science 375, 437–441 (2022).
- Y. Li and M. Koshino, “Twist-angle dependence of the proximity spin-orbit coupling in graphene on transition-metal dichalcogenides,” Phys. Rev. B 99, 075438 (2019).
- S. Chen, M. He, Y.-H. Zhang, V. Hsieh, Z. Fei, K. Watanabe, T. Taniguchi, D. H. Cobden, X. Xu, C. R. Dean, and M. Yankowitz, “Electrically tunable correlated and topological states in twisted monolayer–bilayer graphene,” Nature Physics 17, 374–380 (2021).
- H. Polshyn, J. Zhu, M. A. Kumar, Y. Zhang, F. Yang, C. L. Tschirhart, M. Serlin, K. Watanabe, T. Taniguchi, A. H. MacDonald, and A. F. Young, “Electrical switching of magnetic order in an orbital chern insulator,” Nature 588, 66–70 (2020).
- J. M. Park, Y. Cao, K. Watanabe, T. Taniguchi, and P. Jarillo-Herrero, “Tunable strongly coupled superconductivity in magic-angle twisted trilayer graphene,” Nature 590, 249–255 (2021).
- H. Kim, Y. Choi, C. Lewandowski, A. Thomson, Y. Zhang, R. Polski, K. Watanabe, T. Taniguchi, J. Alicea, and S. Nadj-Perge, “Evidence for unconventional superconductivity in twisted trilayer graphene,” Nature 606, 494–500 (2022).
- X. Liu, Z. Hao, E. Khalaf, J. Y. Lee, Y. Ronen, H. Yoo, D. Haei Najafabadi, K. Watanabe, T. Taniguchi, A. Vishwanath, and P. Kim, “Tunable spin-polarized correlated states in twisted double bilayer graphene,” Nature 583, 221–225 (2020).
- G. W. Burg, J. Zhu, T. Taniguchi, K. Watanabe, A. H. MacDonald, and E. Tutuc, “Correlated insulating states in twisted double bilayer graphene,” Phys. Rev. Lett. 123, 197702 (2019).
- M. He, Y. Li, J. Cai, Y. Liu, K. Watanabe, T. Taniguchi, X. Xu, and M. Yankowitz, “Symmetry breaking in twisted double bilayer graphene,” Nature Physics 17, 26–30 (2021).
- Y. Cao, D. Rodan-Legrain, O. Rubies-Bigorda, J. M. Park, K. Watanabe, T. Taniguchi, and P. Jarillo-Herrero, “Tunable correlated states and spin-polarized phases in twisted bilayer–bilayer graphene,” Nature 583, 215–220 (2020).
- F. Haddadi, Q. Wu, A. J. Kruchkov, and O. V. Yazyev, “Moiré flat bands in twisted double bilayer graphene,” Nano Letters 20, 2410–2415 (2020).
- P. C. Adak, S. Sinha, U. Ghorai, L. D. V. Sangani, K. Watanabe, T. Taniguchi, R. Sensarma, and M. M. Deshmukh, “Tunable bandwidths and gaps in twisted double bilayer graphene on the verge of correlations,” Phys. Rev. B 101, 125428 (2020).
- C. Zhang, T. Zhu, S. Kahn, S. Li, B. Yang, C. Herbig, X. Wu, H. Li, K. Watanabe, T. Taniguchi, S. Cabrini, A. Zettl, M. P. Zaletel, F. Wang, and M. F. Crommie, “Visualizing delocalized correlated electronic states in twisted double bilayer graphene,” Nature Communications 12, 2516 (2021).
- F. Wu, T. Lovorn, E. Tutuc, I. Martin, and A. H. MacDonald, “Topological insulators in twisted transition metal dichalcogenide homobilayers,” Phys. Rev. Lett. 122, 086402 (2019).
- L. Wang, E.-M. Shih, A. Ghiotto, L. Xian, D. A. Rhodes, C. Tan, M. Claassen, D. M. Kennes, Y. Bai, B. Kim, K. Watanabe, T. Taniguchi, X. Zhu, J. Hone, A. Rubio, A. N. Pasupathy, and C. R. Dean, “Correlated electronic phases in twisted bilayer transition metal dichalcogenides,” Nature Materials 19, 861–866 (2020).
- G. Chen, L. Jiang, S. Wu, B. Lyu, H. Li, B. L. Chittari, K. Watanabe, T. Taniguchi, Z. Shi, J. Jung, Y. Zhang, and F. Wang, “Evidence of a gate-tunable mott insulator in a trilayer graphene moiré superlattice,” Nature Physics 15, 237–241 (2019).
- G. Chen, A. L. Sharpe, E. J. Fox, Y.-H. Zhang, S. Wang, L. Jiang, B. Lyu, H. Li, K. Watanabe, T. Taniguchi, Z. Shi, T. Senthil, D. Goldhaber-Gordon, Y. Zhang, and F. Wang, “Tunable correlated chern insulator and ferromagnetism in a moiré superlattice,” Nature 579, 56–61 (2020).
- N. R. Chebrolu, B. L. Chittari, and J. Jung, “Flat bands in twisted double bilayer graphene,” Phys. Rev. B 99, 235417 (2019).
- M. Koshino, “Band structure and topological properties of twisted double bilayer graphene,” Phys. Rev. B 99, 235406 (2019).
- C. L. Kane and E. J. Mele, “Quantum spin hall effect in graphene,” Phys. Rev. Lett. 95, 226801 (2005a).
- C. L. Kane and E. J. Mele, “Topological order and the quantum spin hall effect,” Phys. Rev. Lett. 95, 146802 (2005b).
- M. Ezawa, “A topological insulator and helical zero mode in silicene under an inhomogeneous electric field,” New Journal of Physics 14, 033003 (2012a).
- P. Moon, Y.-W. Son, and M. Koshino, “Optical absorption of twisted bilayer graphene with interlayer potential asymmetry,” Phys. Rev. B 90, 155427 (2014b).
- P. Mohan, U. Ghorai, and R. Sensarma, “Trional warping, satellite dirac points, and multiple field tuned topological transitions in twisted double bilayer graphene,” Phys. Rev. B 103, 155149 (2021).
- E. McCann, “Electronic properties of monolayer and bilayer graphene,” in Graphene Nanoelectronics (Springer Berlin Heidelberg, 2011) pp. 237–275.
- S. Dai, Y. Xiang, and D. J. Srolovitz, “Twisted bilayer graphene: Moiré with a twist,” Nano Letters 16, 5923–5927 (2016).
- T. Fukui, Y. Hatsugai, and H. Suzuki, “Chern numbers in discretized brillouin zone: Efficient method of computing (spin) hall conductances,” Journal of the Physical Society of Japan 74, 1674–1677 (2005).
- M. Ezawa, “Quasi-topological insulator and trigonal warping in gated bilayer silicene,” Journal of the Physical Society of Japan 81, 104713 (2012b).
- P. Mohan and S. Rao, “Interplay of floquet lifshitz transitions and topological transitions in bilayer dirac materials,” Phys. Rev. B 98, 165406 (2018).
- Z. Li, J. Zhuang, L. Chen, Z. Ni, C. Liu, L. Wang, X. Xu, J. Wang, X. Pi, X. Wang, Y. Du, K. Wu, and S. X. Dou, “Observation of van hove singularities in twisted silicene multilayers,” ACS Central Science 2, 517–521 (2016).
- G. Han, H. Shan, L. Zhang, W. Xu, Z.-Y. Gao, H. Guo, G. Li, and H.-J. Gao, “Construction of twisted graphene-silicene heterostructures,” Nano Research 16, 7926–7930 (2023).
- P. Bampoulis, C. Castenmiller, D. J. Klaassen, J. van Mil, Y. Liu, C.-C. Liu, Y. Yao, M. Ezawa, A. N. Rudenko, and H. J. W. Zandvliet, “Quantum spin hall states and topological phase transition in germanene,” Phys. Rev. Lett. 130, 196401 (2023).
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