Quantised helicity in optical media

Abstract: Optical helicity quantifies the handedness of light, and plays a central role in the description of interactions between light and chiral matter. In free space, it is related to the duality symmetry of the electromagnetic field, a continuous symmetry encapsulating the invariance of Maxwell's equations under the interchange of electric and magnetic fields. However, in materials the situation is not so straightforward, as the free space transformation must be extended to encompass mixing of both the $\mathbf{E}$/$\mathbf{H}$ and $\mathbf{D}$/$\mathbf{B}$ field pairs. The simultaneous direct interchange of $\mathbf{E}$/$\mathbf{H}$ and of $\mathbf{D}$/$\mathbf{B}$ is incompatible with the presence of linear constitutive relations. In this work, we extend the duality transform in a way that resolves this incompatibility, and use this to define the optical helicity in a general medium, which may be dispersive, lossy, chiral or nonreciprocal. We find that the helicity density must contain an explicit contribution associated with the polarisation and magnetisation of the matter, and we show that the form of this matter contribution is independent of the details of the medium. We also show that the in-medium helicity can be naturally expressed in terms of the elementary quantised excitations of the system.