One-dimensional Photonic Crystal Structure Enhanced External-Magnetic-Field-Free Spintronic Terahertz High-Field Emitter

Abstract: Intense terahertz (THz) radiation in free space offers multifaceted capabilities for accelerating electron, understanding the mesoscale architecture in (bio)materials, elementary excitation and so on. Recently popularized spintronic THz emitters (STEs) with their versatility such as ultra-broadband, cost-effectiveness, large-size and ease for-integration have become one of the most promising alternative for the next generation of intense THz sources. Nevertheless, the typical W| Co20Fe60B20 | Pt necessitates an external-magnetic-field to saturate magnetization for stable operation, limiting its scalability for achieving higher THz field with uniform distribution over larger sample areas. Here we demonstrate the methodologies of enhancing the high-field THz radiation of external-magnetic-field-free IrMn3 | Co20Fe60B20 |W heterostructure via optimizing the substrate with superior thermal conductivity and integrating a one-dimensional photonic crystal (PC) structure to maximize the radiation efficiency. Under the excitation of a Ti: sapphire femtosecond laser amplifier with central wavelength of 800 nm, pulse duration of 35 fs, and repetition rate of 1 kHz and maximum single pulse energy of 5.5 mJ, we successfully generate intense THz radiation with focal peak electric field up to 1.1 MV/cm with frequency range covering 0.1-10 THz without external-magnetic-fields. These high-field STEs will also enable other applications such as ultra-broadband high-field THz spectroscopy and polarization-based large-size strong-field THz imaging.