Electronic anisotropy and rotational symmetry breaking at a Weyl semimetal/spin ice interface

Abstract: In magnetic pyrochlore materials, the interplay of spin-orbit coupling, electronic correlations, and geometrical frustration gives rise to exotic quantum phases, including topological semimetals and spin ice. While these phases have been observed in isolation, the interface-driven phenomena emerging from their interaction have never been realized previously. Here, we report on the discovery of interfacial electronic anisotropy and rotational symmetry breaking at a heterostructure consisting of the Weyl semimetal Eu2Ir2O7 and spin ice Dy2Ti2O7. Subjected to magnetic fields, we unveil a six-fold anisotropic transport response that is theoretically accounted by a Kondo-coupled heterointerface, where the spin ice's field-tuned magnetism induces electron scattering in the Weyl semimetal's topological Fermi-arc states. Furthermore, at elevated magnetic fields, we reveal a two-fold anisotropic response indicative of a new symmetry-broken many-body state. This discovery showcases the nascent potential of complex quantum architectures in search of emergent phenomena unreachable in bulk crystals.