Non-linear anomalous Edelstein response at altermagnetic interfaces

Abstract: In altermagnets, time-reversal symmetry breaking spin-polarizes electronic states, while total magnetization remains zero. In addition, at altermagnetic surfaces Rashba-spin orbit coupling is activated due to broken inversion symmetry, introducing a competing spin-momentum locking interaction. Here we show that their interplay leads to the formation of complex, chiral spin textures that offer novel, non-linear spin-to-charge conversion properties. Whereas altermagnetic order suppresses the canonical linear in-plane Rashba-Edelstein response, we establish the presence of an anomalous transversal Edelstein effect for planar applied electric and magnetic field, or alternatively, an in-plane magnetization. Moreover the non-linear Edelstein response resulting purely from electric fields also triggers the anomalous out-of-plane magnetization. We determine the anomalous response with a model based on the ab-initio electronic structure of RuO$_2$ bilayers, ultimately opening experimental avenues to explore spin-charge conversion phenomena at altermagnetic interfaces.