Gyrotropic Magnetic Effect in Black Phosphorus Irradiated with Bicircular Light

Abstract: The gyrotropic magnetic effect, manifesting as a gyropropic current under a slowly-varying magnetic field, represents a fundamental property of Bloch electrons on the Fermi surface; however, it has not been observed in experiments. Here, we theoretically propose that Floquet engineering with bicircular light (BCL), which is a superposition of two opposite chiral waves of circularly polarized light with an integer frequency ratio, presents a fascinating strategy to generate and manipulate the gyrotropic magnetic effect in nodal line semimetals. The tailoring spatial symmetry of BCL irradiation can induce a topological transition from a nodal line semimetallic phase to a Weyl semimetallic phase characterized by a minimum number of misaligned Weyl nodes, resulting in the generation of gyrotropic current when a slowly oscillating magnetic field is applied. Moreover, using first-principles calculations, we show that the compressed black phosphorus under irradiation of BCL is an ideal candidate to realize the large gyropropic current with great advantages. Our work not only broadens potential candidate materials for achieving the experimentally accessible gyropropic current, but also provides deeper insights into the interplay between topological phenomena and light manipulation of symmetries.