Resonant second harmonic generation in a two-dimensional electron system

Abstract: We consider the nonlinear response of a disordered two-dimensional electronic system, lacking inversion symmetry, to an external alternating electric field. The application of an in-plane static magnetic field induces local contributions to the current density that are quadratic in the electric field and linear in the magnetic field. This current oscillates at twice the frequency of the external irradiation and there are two linearly independent vector combinations that contribute to the current density. This particular mechanism coexists with the topological Berry-dipole contribution to the second harmonic of the current density, which can be generated by quantum confinement. Additional nonlocal terms in the current density are possible in the regime away from the normal incidence. The total current exhibits a nonreciprocal character upon reversal of the magnetic field direction. We evaluate the magnitude of this effect by computing its dependence on the strength of spin-orbit coupling and the disorder scattering rate. Importantly, we show that these local second-harmonic contributions can be resonantly excited when the frequency of the external radiation approaches the energy separation between the spin-orbit split bands.