Enhanced quantum frequency estimation by nonlinear scrambling

Abstract: Frequency estimation, a cornerstone of basic and applied sciences, has been significantly enhanced by quantum sensing strategies. Despite breakthroughs in quantum-enhanced frequency estimation, key challenges remain: static probes limit flexibility, and the interplay between resource efficiency, sensing precision, and potential enhancements from nonlinear probes remains not fully understood. In this work, we show that dynamically encoding an unknown frequency in a nonlinear quantum electromagnetic field can significantly improve frequency estimation. To provide a fair comparison of resources, we define the energy cost as the figure of merit for our sensing strategy. We further show that specific higher-order nonlinear processes lead to nonlinear-enhanced frequency estimation. This enhancement results from quantum scrambling, where local quantum information spreads across a larger portion of the Hilbert space. We quantify this effect using the Wigner-Yanase skew information, which measures the degree of noncommutativity in the Hamiltonian structure. Our work sheds light on the connection between Wigner-Yanase skew information and quantum sensing, providing a direct method to optimize nonlinear quantum probes.