Discovery of a Highly Anisotropic Type-II Ferromagnetic Weyl State Exhibiting a 3D Quantum Hall Effect

Abstract: Topological semimetals, particularly Weyl semimetals (WSMs), are crucial platforms for exploring emergent quantum phenomena due to their unique electronic structures and potential to transition into various topological phases. In this study, we report the discovery of a ferromagnetic (FM) type-II WSM in Mn(Bi1-xSbx)4Te7, which exhibits a remarkable three-dimensional (3D) quantum Hall effect (QHE). By precisely tuning the chemical potential through Sb doping, we obtained samples with the Fermi level near the charge neutrality point for x = ~ 0.27. This was confirmed by spectroscopy measurements (ARPES and STS), and these samples showed strong quantum oscillations along with a key transport signature of a Weyl state - chiral anomaly, and Fermi surface reconstruction driven by FM ordering. Our theoretical analysis indicates that this Weyl state evolves from a parent nodal ring state, where higher-order k-terms split the nodal line into type-II Weyl nodes. The Weyl state exhibits significant anisotropy, characterized by a pronounced reduction in Fermi velocity along the kz-axis, likely accounting for the observed 3D QHE. These results not only highlight the exceptional tunability of the Mn(Bi1-xSbx)4Te7 system, where precise control of the chemical potential and magnetic properties opens access to novel quantum phases, but also advance the understanding of FM WSMs.