Transient Chirality in the Gelation of Adhesive Spinner Monolayers

Abstract: Active systems of self-rotating elements inherently exhibit chirality, making them of fundamental interest due to parity violation. Using large-scale hydrodynamic simulations, we investigate the gelation of adhesive spinners confined to quasi-2D monolayers at low Reynolds numbers. Unlike the coarsening dynamics of passive colloids, spinner gelation follows a different pathway, displaying structural chirality during the early stages of aggregation. However, this chirality dissipates upon dynamical arrest, resulting in a final gel structure that resembles a conventional colloidal gel. As a result, we find no sign of odd mechanical responses. Nonetheless, the elastic modulus and gelation time remain tunable through spinning activity, providing a new avenue for the bottom-up design of programmable soft materials.