Observing Spatial Charge and Spin Correlations in a Strongly-Interacting Fermi Gas

Abstract: Two-dimensional correlated fermions constitute a cornerstone of quantum matter, covering a broad fundamental and technological scope, and have attracted increasing interest with the emergence of modern materials such as high-$T_{\rm c}$ superconductors, graphene, topological insulators, and Moir\'e structures. Atom-based quantum simulators provide a new pathway to understand the microscopic mechanisms occurring at the heart of such systems. In this work, we explore two-dimensional attractive Fermi gases at the microscopic level by probing spatial charge and spin correlations in situ. Using atom-resolved continuum quantum gas microscopy, we directly observe fermion pairing and study the evolution of two- and three-point correlation functions as inter-spin attraction is increased. The precision of our measurement allows us to reveal a marked dip in the pair correlation function, fundamentally forbidden by the mean-field result based on Bardeen-Cooper-Schrieffer (BCS) theory but whose existence we confirm in exact auxiliary-field quantum Monte Carlo calculations. We demonstrate that the BCS prediction is critically deficient not only in the superfluid crossover regime but also deep in the weakly attractive side. Guided by our measurements, we find a remarkable relation between two- and three-point correlations that establishes the dominant role of pair-correlations. Finally, leveraging local single-pair losses, we independently characterize the short-range behavior of pair correlations, via the measurement of Tan's Contact, and find excellent agreement with numerical predictions. Our measurements provide an unprecedented microscopic view into two-dimensional Fermi gases and constitute a paradigm shift for future studies of strongly-correlated fermionic matter in the continuum.