Elastic instability of wormlike micelle solution flow in serpentine channels

Abstract: Wormlike micelle (WLM) solutions are abundant in energy, environmental, and industrial applications, which often rely on their flow through tortuous channels. How does the interplay between fluid rheology and channel geometry influence the flow behavior? Here, we address this question by experimentally visualizing and quantifying the flow of a semi-dilute WLM solution in millifluidic serpentine channels. At low flow rates, the base flow is steady and laminar, with strong asymmetry and wall slip. When the flow rate exceeds a critical threshold, the flow exhibits an elastic instability, producing spatially-heterogeneous, unsteady three-dimensional (3D) flow characterized by two notable features: (i) the formation and persistence of stagnant but strongly-fluctuating and multistable "dead zones" in channel bends, and (ii) intermittent 3D "twists" throughout the bulk flow. The geometry of these dead zones and twisting events can be rationalized by considering the minimization of local streamline curvature to reduce flow-generated elastic stresses. Altogether, our results shed new light into how the interplay between solution rheology and tortuous boundary geometry influences WLM flow behavior, with implications for predicting and controlling WLM flows in a broad range of complex environments.