Diverse electronic phases correlated with twist-angle distribution and pseudomagnetic field in turbostratic graphene

Abstract: Twisted multilayer graphene has become a focal point of research due to its ability to host a range of quantum phases, including unconventional superconductivity, ferromagnetism, and strong correlation effects. In the present work, we address the challenge of investigating the diverse physics associated with a variety of twist-angles in a simple graphene platform which is economic and bypasses the tedious process of fabricating multiple devices, each with one twist angle. We used turbostratic graphene films containing a variety of twist angles characterized by distinct Moir\'e patterns observed through scanning tunneling microscopy (STM), and distinct signatures recorded by Raman spectroscopy. From scanning tunneling spectroscopy (STS), we show that the local twist angles remarkably correlate with the characteristic local electronic properties. Most remarkably, the films spontaneously generate strained wrinkles during growth, with certain wrinkled regions exhibiting robust strain-induced pseudo-magnetic fields, as recorded by ultra-low temperature STS.