Current-induced Nonequilibrium Phase Transition Accompanied by Giant Gap Reduction in Vanadium Dioxide

Abstract: We investigated nonlinear conduction in bulk single crystals of VO2 with precise temperature control. Two distinct nonequilibrium phenomena were identified: a gradual reduction of the charge gap and a current-induced insulator-metal transition. The electric field required to drive the nonlinear conduction is two to three orders of magnitude smaller than that reported for VO2 thin films or nanobeams, strongly indicating an intrinsic electronic origin rather than a temperature increase due to self heating. Notably, our results suggest that the application of a steady current to the frozen insulating state can induce a nonequilibrium steady-state metallic phase -- effectively melting the electronic ice. This highlights a novel route to controlling electronic states via nonthermal, current-driven mechanisms.