Unveiling Mechanical Motions in Non-linear Optical Organic Micro Ring Resonators

Abstract: This work demonstrates the multifaceted dynamic motion and three-dimensional (3D) spatial manipulation of organic micro ring resonators (MRRs). The MRRs are fabricated via surface-tension-assisted self-assembly of 2,2'-((1E,1'E)-hydrazine-1,2-diylidenebis(methaneylylidene))bis(3,5-dibromophenol) (HDBP), exhibiting nonlinear optical (NLO) emission and frequency comb-type whispering gallery modes. Interestingly, the MRRs are micromechanically reconfigurable into various strained architectures, including lifting, transferring, vertical standing, axial spinning, and wheel-like rolling, using an atomic force microscopy cantilever tip. The MRRs retained their photonic traits throughout these dynamic motions, underscoring their mechanical robustness. Notably, the demonstration of axial spinning and rolling locomotion extends the manipulation capabilities beyond two-dimensional control, enabling complete 3D spatial control. These results establish a foundational platform for next-generation NLO mechanophotonic systems, where reconfigurable smart and soft photonic elements can be dynamically controlled with high spatial precision.