Ultrafast cooperative electronic, structural, and magnetic switching in an altermagnet

Abstract: Femtosecond laser control of antiferromagnetic order is a cornerstone for future memory and logic devices operating at terahertz clock rates. The advent of altermagnets -- antiferromagnets with unconventional spin-group symmetries -- creates new opportunities in this evolving field. Here, we demonstrate ultrafast laser-induced switching in altermagnetic $\alpha$-MnTe that orchestrates the concerted dynamics of charge, lattice, and spin degrees of freedom. Time-resolved reflectivity and birefringence measurements reveal that the transient melting of spin order is accompanied by pronounced structural and electronic instabilities, as evidenced by phonon nonlinearity and accelerated band gap shrinkage. Theoretical modeling highlights the key roles of robust magnetic correlations and spin-charge coupling pathways intrinsic to this altermagnet.