Advanced creep modelling for polymers: A variable-order fractional calculus approach

Abstract: Polymer-based plastics exhibit time-dependent deformation under constant stress, known as creep, which can lead to rupture or static fatigue. A common misconception is that materials under tolerable static loads remain unaffected over time. Accurate long-term deformation predictions require experimental creep data, but conventional models based on simple rheological elements like springs and dampers often fall short, lacking the flexibility to capture the power-law behaviour intrinsic to creep processes. The springpot, a fractional calculus-based element, has been used to provide a power-law relationship; however, its fixed-order nature limits its accuracy, particularly when the deformation rate evolves over time. This article introduces a variable-order (VO) springpot model that dynamically adapts to the evolving viscoelastic properties of polymeric materials during creep, capturing changes between glassy, transition and rubbery phases. Model parameters are calibrated using a robust procedure for model identification based on the cross-entropy (CE) method, resulting in physically consistent and accurate predictions. This advanced modelling framework not only overcomes the limitations of the fixed-order models but also establishes a foundation for applying VO mechanics to other viscoelastic materials, providing a valuable tool for predicting long-term material performance in structural applications.