Terahertz Attoclock

Abstract: The attoclock provides a powerful tool for studying ultrafast electron dynamics on the attosecond timescale. We demonstrate an all-optical terahertz (THz) attoclock that reconstructs electron dynamics during photoionization by detecting THz radiation emitted from gases ionized by the fundamental and second harmonic two-color laser fields, without the need for photoelectron detection. The polarization direction of the emitted THz field reflects the direction of the photoelectron drift velocity and thus encodes the effective delay. By measuring the THz waves from argon atoms ionized by the two-color fields, and by precisely controlling their relative phase and ellipticity, we observe intensity-dependent rotations of the THz polarization direction. Both experiment and time-dependent Schrodinger equation simulations reveal that the effective delay extracted from the THz polarization direction decreases with increasing laser intensity, consistent with conventional photoelectron attoclock results. Our experiment establishes the feasibility of the THz attoclock as a contactless probe of tunneling dynamics, with promising applications to condensed matter systems where photoelectron detection is impractical.