Terahertz Emission from Spintronic Stack Nanodecorated with Drop-Cast Core-Shell Plasmonic Nanoparticles

Abstract: Spintronic emitters promise to revolutionise terahertz (THz) sources by converting ultrafast optical pulses into broadband THz radiation without phase-matching constraints. Because the conversion relies on spin-current injection across a nanometre-thin magnetic layer, its efficiency is ordinarily limited by weak optical coupling. Here, we present a demonstration of a drop-casting based approach to introduce ultrafast plasmonic-mediated coupling: a sparse-layer of silica-gold core-shell nanoparticles is deposited directly onto a W/Fe/Pt spintronic trilayer. This sparse (six percent) decoration increases the wafer-averaged THz pulse energy, pointing to a very high local conversion enhancement for this low-coverage spintronic emitter compared with the bare stack. This demonstration points to a viable pathway toward highly efficient spintronic terahertz emitters with potential applications in spectroscopy, imaging, and ultrafast technologies.