Robust photon blockade with hybrid molecular optomechanics

Abstract: Molecular cavity optomechanical systems, featuring ultrahigh vibrational frequencies and strong light-matter interactions, hold significant promise for advancing applications in quantum science and technology. Specifically, by introducing metallic nanoparticles into microcavities, hybrid molecular cavity optomechanical systems can further enhance optical quality factors and system tunabilities, which enables scalable and controllable quantum platforms. In this study, we propose how to realize robust photon blockade, i.e., strong photon antibunching with arbitrary detuning conditions, by combining degenerate optical parametric amplification with a hybrid molecular cavity optomechanical system. More interesting, we find near-perfect optomechanical photon blockade at room temperature, which is robust against temperature and optical dissipation. In addition, our approach can release the strict condition of high temporal resolution by combining features of conventional and unconventional photon blockade. Our approach offers a feasible route to study intriguing quantum effects in hybrid molecular cavity optomechanical systems, and holds promise for applications in nonclassical state engineering, quantum sensing, and photonic precision measurements.